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Near-neutral-colored semitransparent perovskite films using a combination of colloidal self-assembly and plasma etching

Zhang, Lijing, Hörantner, Maximilian T., Zhang, Wei, Yan, Qingfeng and Snaith, Henry J. (2016) Near-neutral-colored semitransparent perovskite films using a combination of colloidal self-assembly and plasma etching Solar Energy Materials and Solar Cells, 160. pp. 193-202.

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Abstract

Organo-lead-halide perovskite based solar cells have achieved remarkable advancements in power conversion efficiencies (PCEs) in recent years. Given their attractive properties, possible applications for perovskites are wide ranging and among others, particularly appealing for building integrated photovoltaics (BIPVs). In this study, patterned perovskite films were successfully fabricated based on a microsphere lithography SiO2 honeycomb scaffold template, which was derived by a combination of air-water interface self-assembly and O2 plasma etching. These patterned perovskite films exhibited near-neutral-color and tunable semitransparency, which meet the requisites of semitransparent solar cells for BIPVs application. O2 plasma etching of the microsphere template could effectively improve the active layer average visible transmission (AVT), and the existence of the SiO2 nanoscaffold effectively smoothed the internal trade-off of active layer AVT and device PCE. Solar cell devices fabricated with these optimized patterened perovskite films yielded a maximum PCE of 10.3% with relatively high active layer AVT of 38%. This nanoscaffold patterned perovskite opens up a new strategy for design and fabrication of functional photoelectric device based on organo-lead-halide perovskite.

Item Type: Article
Divisions : Faculty of Engineering and Physical Sciences > Electronic Engineering
Authors :
NameEmailORCID
Zhang, LijingUNSPECIFIEDUNSPECIFIED
Hörantner, Maximilian T.UNSPECIFIEDUNSPECIFIED
Zhang, Weiwz0003@surrey.ac.ukUNSPECIFIED
Yan, QingfengUNSPECIFIEDUNSPECIFIED
Snaith, Henry J.UNSPECIFIEDUNSPECIFIED
Date : 28 October 2016
Identification Number : https://doi.org/10.1016/j.solmat.2016.10.035
Copyright Disclaimer : © 2016. This manuscript version is made available under the CC-BY-NC-ND 4.0 license http://creativecommons.org/licenses/by-nc-nd/4.0/
Uncontrolled Keywords : Semi-transparent; Perovskite films; Solar cell; Colloidal crystal; Nanoscaffold
Depositing User : Clive Harris
Date Deposited : 05 Jun 2017 13:14
Last Modified : 13 Jun 2017 13:22
URI: http://epubs.surrey.ac.uk/id/eprint/841295

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