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Plasmonic-Induced Photon Recycling in Metal Halide Perovskite Solar Cells

Saliba, Michael, Zhang, Wei, Burlakov, Victor M., Stranks, Samuel D., Sun, Yao, Ball, James M., Johnston, Michael B., Goriely, Alain, Wiesner, Ulrich and Snaith, Henry J. (2015) Plasmonic-Induced Photon Recycling in Metal Halide Perovskite Solar Cells Advanced Functional Materials, 25 (31). pp. 5038-5046.

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Abstract

Organic–inorganic metal halide perovskite solar cells have emerged in the past few years to promise highly efficient photovoltaic devices at low costs. Here, temperature-sensitive core–shell Ag@TiO2 nanoparticles are successfully incorporated into perovskite solar cells through a low-temperature processing route, boosting the measured device efficiencies up to 16.3%. Experimental evidence is shown and a theoretical model is developed which predicts that the presence of highly polarizable nanoparticles enhances the radiative decay of excitons and increases the reabsorption of emitted radiation, representing a novel photon recycling scheme. The work elucidates the complicated subtle interactions between light and matter in plasmonic photovoltaic composites. Photonic and plasmonic schemes such as this may help to move highly efficient perovskite solar cells closer to the theoretical limiting efficiencies.

Item Type: Article
Divisions : Faculty of Engineering and Physical Sciences > Electronic Engineering
Authors :
NameEmailORCID
Saliba, MichaelUNSPECIFIEDUNSPECIFIED
Zhang, Weiwz0003@surrey.ac.ukUNSPECIFIED
Burlakov, Victor M.UNSPECIFIEDUNSPECIFIED
Stranks, Samuel D.UNSPECIFIEDUNSPECIFIED
Sun, YaoUNSPECIFIEDUNSPECIFIED
Ball, James M.UNSPECIFIEDUNSPECIFIED
Johnston, Michael B.UNSPECIFIEDUNSPECIFIED
Goriely, AlainUNSPECIFIEDUNSPECIFIED
Wiesner, UlrichUNSPECIFIEDUNSPECIFIED
Snaith, Henry J.UNSPECIFIEDUNSPECIFIED
Date : 19 August 2015
Funders : Engineering and Physical Sciences Research Council, EPSRC
Identification Number : 10.1002/adfm.201500669
Copyright Disclaimer : © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Uncontrolled Keywords : Perovskite solar cells; Core–shell nanoparticles; Plasmonics
Depositing User : Clive Harris
Date Deposited : 01 Jun 2017 09:46
Last Modified : 05 Jun 2017 09:39
URI: http://epubs.surrey.ac.uk/id/eprint/841260

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