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Strategies for carbon and sulfur tolerant solid oxide fuel cell materials, incorporating lessons from heterogeneous catalysis

Boldrin, P, Ruiz-Trejo, E, Mermelstein, J, Bermudez Menendez, J, Ramirez Reina, T and Brandon, NP (2016) Strategies for carbon and sulfur tolerant solid oxide fuel cell materials, incorporating lessons from heterogeneous catalysis Chemical Reviews.

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Abstract

Solid oxide fuel cells (SOFCs) are a rapidly emerging energy technology for a low carbon world, providing high efficiency, potential to use carbonaceous fuels and compatibility with carbon capture and storage. However, current state-of-the-art materials have low tolerance to sulfur, a common contaminant of many fuels, and are vulnerable to deactivation due to carbon deposition when using carbon-containing compounds. In this review we first study the theoretical basis behind carbon and sulfur poisoning, before examining the strategies towards carbon and sulfur tolerance used so far in the SOFC literature. We then study the more extensive relevant heterogeneous catalysis literature for strategies and materials which could be incorporated into carbon and sulfur tolerant fuel cells.

Item Type: Article
Subjects : Chemical and Process Engineering
Divisions : Faculty of Engineering and Physical Sciences > Chemical and Process Engineering
Authors :
NameEmailORCID
Boldrin, PUNSPECIFIEDUNSPECIFIED
Ruiz-Trejo, EUNSPECIFIEDUNSPECIFIED
Mermelstein, JUNSPECIFIEDUNSPECIFIED
Bermudez Menendez, JUNSPECIFIEDUNSPECIFIED
Ramirez Reina, TUNSPECIFIEDUNSPECIFIED
Brandon, NPUNSPECIFIEDUNSPECIFIED
Date : 9 November 2016
Identification Number : 10.1021/acs.chemrev.6b00284
Copyright Disclaimer : This document is the Accepted Manuscript version of a Published Work that appeared in final form in Chemical Reviews, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see http://pubs.acs.org/doi/abs/10.1021/acs.chemrev.6b00284
Depositing User : Symplectic Elements
Date Deposited : 26 Oct 2016 12:00
Last Modified : 09 Nov 2017 02:09
URI: http://epubs.surrey.ac.uk/id/eprint/812621

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