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Nucleation of a new phase on a surface that is changing irreversibly with time

Sear, Richard (2014) Nucleation of a new phase on a surface that is changing irreversibly with time Physical Review E: Statistical, Nonlinear, and Soft Matter Physics, 89.

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Abstract

Nucleation of a new phase almost always starts at a surface. This surface is almost always assumed not to change with time. However, surfaces can roughen, partially dissolve and change chemically with time. Each of these irreversible changes will change the nucleation rate at the surface, resulting in a time-dependent nucleation rate. Here we use a simple model to show that partial surface dissolution can qualitatively change the nucleation process, in a way that is testable in experiment. The changing surface means that the nucleation rate is increasing with time. There is an initial period during which no nucleation occurs, followed by relatively rapid nucleation.

Item Type: Article
Divisions : Faculty of Engineering and Physical Sciences > Physics
Authors :
NameEmailORCID
Sear, RichardR.Sear@surrey.ac.ukUNSPECIFIED
Date : 2 January 2014
Identification Number : 10.1103/PhysRevE.89.022405
Copyright Disclaimer : Published by the American Physical Society under the terms of the Creative Commons Attribution 3.0 License. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI
Depositing User : Symplectic Elements
Date Deposited : 01 May 2014 09:25
Last Modified : 26 Jul 2017 09:08
URI: http://epubs.surrey.ac.uk/id/eprint/805478

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